Portuguese is spoken in relatively few countries, but they are located throughout the world. The country with the largest Portuguese speaking population isn’t Portugal, rather it is a country across the Atlantic and in the Southern Hemisphere. That country is of course Brazil with over 202 million. Then two Sub-Saharan African countries of Mozambique and Angola each have around 24 million each and with Portugal having 10 million, it is the 4th largest Portuguese speaking population.